TY - JOUR
T1 - Very low temperature electronic transport in Al-Pd-Re quasicrystalline alloys
AU - Rosenbaum, Ralph
AU - Balanetskyy, Sergiy
AU - Grushko, Benjamin
AU - Przepiórzyński, Bartosz
N1 - Funding Information:
Acknowledgements We thank C. Thomas and W. Reichert for technical contributions at the Forsch-ungszentrum Jülich and Drs. Tim Murphy and Eric Palm at the NHMFL. We are obliged to Drs. V. Shemet and A. Gil at the Forschungszentrum Jülich for discussions on oxidation processes. We are indebted to Mrs. R. Rosenbaum for editorial assistance. A portion of this work was performed at the National High Magnetic Field Laboratory (NHMFL), which is supported by NSF Cooperative Agreement No. DMR-0084173, by the State of Florida and by the DOE.
PY - 2008/1
Y1 - 2008/1
N2 - Electrical resistivities of two icosahedral (I) Al-Pd-Re alloys have been measured between room temperature and mK temperatures. One quasicrystalline (QC) polygrain Al-Pd-Re sample exhibited insulating behavior in its resistivities, increasing by a factor of r = R (4 K)/R (300 K)=7.76; its room temperature resistivity was 9,890 μΩcm. A "phenomenological" expression fitted the conductivity data well between 300 K to 0.5 K. Below 0.4 K a crossover to an activated variable-range hopping law was observed. Low temperature magnetoresistance ratio data and fits using the wave function shrinkage theory are presented. A second QC Al-Pd-Re sample had a small resistance temperature ratio r = 2.12. The room temperature resistivity was extremely large, ρ(300 K)≈40,980 μΩcm. Its conductivity could be described well using a simple temperature power law between 300 K to 20 K. Below 20 K there was a crossover to a new behavior. Below 1 K, the conductivity could be fitted using a very weakly insulating power law where σ (T)≈11.37T 0.032 in (Ωcm) -1, suggesting that this sample is located just below the metal-insulator transition. The magnetoconductivity data could not be fitted successfully using the 3D weak localization (WL) theory and inserting into it physical and realistic fitting magnitudes for the inelastic magnetic field B in.
AB - Electrical resistivities of two icosahedral (I) Al-Pd-Re alloys have been measured between room temperature and mK temperatures. One quasicrystalline (QC) polygrain Al-Pd-Re sample exhibited insulating behavior in its resistivities, increasing by a factor of r = R (4 K)/R (300 K)=7.76; its room temperature resistivity was 9,890 μΩcm. A "phenomenological" expression fitted the conductivity data well between 300 K to 0.5 K. Below 0.4 K a crossover to an activated variable-range hopping law was observed. Low temperature magnetoresistance ratio data and fits using the wave function shrinkage theory are presented. A second QC Al-Pd-Re sample had a small resistance temperature ratio r = 2.12. The room temperature resistivity was extremely large, ρ(300 K)≈40,980 μΩcm. Its conductivity could be described well using a simple temperature power law between 300 K to 20 K. Below 20 K there was a crossover to a new behavior. Below 1 K, the conductivity could be fitted using a very weakly insulating power law where σ (T)≈11.37T 0.032 in (Ωcm) -1, suggesting that this sample is located just below the metal-insulator transition. The magnetoconductivity data could not be fitted successfully using the 3D weak localization (WL) theory and inserting into it physical and realistic fitting magnitudes for the inelastic magnetic field B in.
KW - Al-Pd-Re phases
KW - Electrical conductivity and resistivity
KW - Insulators
KW - Magnetoresistance
KW - Quasicrystals
UR - http://www.scopus.com/inward/record.url?scp=37549033183&partnerID=8YFLogxK
U2 - 10.1007/s10909-007-9518-3
DO - 10.1007/s10909-007-9518-3
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AN - SCOPUS:37549033183
SN - 0022-2291
VL - 150
SP - 82
EP - 100
JO - Journal of Low Temperature Physics
JF - Journal of Low Temperature Physics
IS - 1-2
ER -