Strain engineering magnetic frustration in perovskite oxide thin films

Carlos Escorihuela-Sayalero*, Oswaldo Diéguez, Jorge Íñiguez

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

38 Scopus citations

Abstract

Our first-principles results show that geometric frustration can be induced in thin films of multiferroic BiFeO3. We find that competing magnetic interactions occur in the so-called supertetragonal phase of this material, which can be grown on strongly compressive substrates. We show that the frustration level can be tuned by appropriately choosing the substrate; in fact, the phase diagram of the films presents a critical line at which the three-dimensional spin order gets annihilated. We argue that these effects are not exclusive to BiFeO3 and predict that they also occur in BiCoO3.

Original languageEnglish
Article number247202
JournalPhysical Review Letters
Volume109
Issue number24
DOIs
StatePublished - 10 Dec 2012
Externally publishedYes

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