Steady-state theory of current transfer

Vered Ben-Moshe; Abraham Nitzan; Spiros S. Skourtis; David N. Beratan

doi:10.1021/jp100661f

Steady-state theory of current transfer

Vered Ben-Moshe, Abraham Nitzan^*, Spiros S. Skourtis, David N. Beratan

^*Corresponding author for this work

School of Chemistry

Research output: Contribution to journal › Article › peer-review

Abstract

Current transfer is defined as a charge-transfer process where the transferred charge carries information about its original motion. We have recently suggested that such transfer causes the asymmetry observed in electron transfer induced by circularly polarized light through helical wires. This paper presents the steady-state theory of current transfer within a tight binding model of coupled wires systems. The asymmetry in the system response to a steady current imposed in a particular direction on one of the wires is used to define the efficiency of current transfer.

Original language	English
Pages (from-to)	8005-8013
Number of pages	9
Journal	Journal of Physical Chemistry C
Volume	114
Issue number	17
DOIs	https://doi.org/10.1021/jp100661f
State	Published - 6 May 2010

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10.1021/jp100661f

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abstract = "Current transfer is defined as a charge-transfer process where the transferred charge carries information about its original motion. We have recently suggested that such transfer causes the asymmetry observed in electron transfer induced by circularly polarized light through helical wires. This paper presents the steady-state theory of current transfer within a tight binding model of coupled wires systems. The asymmetry in the system response to a steady current imposed in a particular direction on one of the wires is used to define the efficiency of current transfer.",

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AU - Beratan, David N.

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N2 - Current transfer is defined as a charge-transfer process where the transferred charge carries information about its original motion. We have recently suggested that such transfer causes the asymmetry observed in electron transfer induced by circularly polarized light through helical wires. This paper presents the steady-state theory of current transfer within a tight binding model of coupled wires systems. The asymmetry in the system response to a steady current imposed in a particular direction on one of the wires is used to define the efficiency of current transfer.

AB - Current transfer is defined as a charge-transfer process where the transferred charge carries information about its original motion. We have recently suggested that such transfer causes the asymmetry observed in electron transfer induced by circularly polarized light through helical wires. This paper presents the steady-state theory of current transfer within a tight binding model of coupled wires systems. The asymmetry in the system response to a steady current imposed in a particular direction on one of the wires is used to define the efficiency of current transfer.

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Steady-state theory of current transfer

Abstract

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