Resonance heterodyne optical Kerr effect spectroscopy of population wave packets with intense chirped pulses

Jonathan Segal; Dan Huppert; Boris Fainberg

doi:10.1016/S0022-2313(02)00621-X

Resonance heterodyne optical Kerr effect spectroscopy of population wave packets with intense chirped pulses

Jonathan Segal, Dan Huppert^*, Boris Fainberg

^*Corresponding author for this work

School of Chemistry

Research output: Contribution to journal › Conference article › peer-review

3 Scopus citations

Abstract

We propose a new method for studying the time evolution of population wavepackets in the ground and excited states of a large dye molecule dissolved in polar liquids: resonance heterodyned optical Kerr effect (HOKE) technique with intense chirped pulses. We found a profound effect on both the ground and excited state transient populations using intense positively and negatively chirped pulses. The dump process is very effective when the sample is excited by negatively chirped intense pulses.

Original language	English
Pages (from-to)	669-675
Number of pages	7
Journal	Journal of Luminescence
Volume	102-103
Issue number	SPEC
DOIs	https://doi.org/10.1016/S0022-2313(02)00621-X
State	Published - May 2003
Event	Proceedings of the 2002 International Conference on Luminescence - Budapest, Hungary Duration: 24 Aug 2002 → 29 Aug 2002

Keywords

Coherent control
Femtosecond
Optical Kerr effect

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10.1016/S0022-2313(02)00621-X

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title = "Resonance heterodyne optical Kerr effect spectroscopy of population wave packets with intense chirped pulses",

abstract = "We propose a new method for studying the time evolution of population wavepackets in the ground and excited states of a large dye molecule dissolved in polar liquids: resonance heterodyned optical Kerr effect (HOKE) technique with intense chirped pulses. We found a profound effect on both the ground and excited state transient populations using intense positively and negatively chirped pulses. The dump process is very effective when the sample is excited by negatively chirped intense pulses.",

keywords = "Coherent control, Femtosecond, Optical Kerr effect",

author = "Jonathan Segal and Dan Huppert and Boris Fainberg",

note = "Funding Information: This work was supported by grants from the Israel Science Foundation and James–Franck German–Israel in laser–matter interaction.; Proceedings of the 2002 International Conference on Luminescence ; Conference date: 24-08-2002 Through 29-08-2002",

year = "2003",

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T1 - Resonance heterodyne optical Kerr effect spectroscopy of population wave packets with intense chirped pulses

AU - Segal, Jonathan

AU - Huppert, Dan

AU - Fainberg, Boris

N1 - Funding Information: This work was supported by grants from the Israel Science Foundation and James–Franck German–Israel in laser–matter interaction.

PY - 2003/5

Y1 - 2003/5

N2 - We propose a new method for studying the time evolution of population wavepackets in the ground and excited states of a large dye molecule dissolved in polar liquids: resonance heterodyned optical Kerr effect (HOKE) technique with intense chirped pulses. We found a profound effect on both the ground and excited state transient populations using intense positively and negatively chirped pulses. The dump process is very effective when the sample is excited by negatively chirped intense pulses.

AB - We propose a new method for studying the time evolution of population wavepackets in the ground and excited states of a large dye molecule dissolved in polar liquids: resonance heterodyned optical Kerr effect (HOKE) technique with intense chirped pulses. We found a profound effect on both the ground and excited state transient populations using intense positively and negatively chirped pulses. The dump process is very effective when the sample is excited by negatively chirped intense pulses.

KW - Coherent control

KW - Femtosecond

KW - Optical Kerr effect

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SN - 0022-2313

VL - 102-103

SP - 669

EP - 675

JO - Journal of Luminescence

JF - Journal of Luminescence

IS - SPEC

T2 - Proceedings of the 2002 International Conference on Luminescence

Y2 - 24 August 2002 through 29 August 2002

ER -

Resonance heterodyne optical Kerr effect spectroscopy of population wave packets with intense chirped pulses

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Keywords

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