Relaxation of excess electrons in a polar solvent

P. M. Rentzepis; R. P. Jones; Joshua Jortner

doi:10.1016/0009-2614(72)80353-1

Relaxation of excess electrons in a polar solvent

P. M. Rentzepis^*, R. P. Jones, Joshua Jortner

^*Corresponding author for this work

School of Chemistry

Lucent

Research output: Contribution to journal › Article › peer-review

35 Scopus citations

Abstract

We report the observation of the ultrafast relaxation of a quasifree electron to the localized excess electron state in water. Quasifree electrons were generated by photoionization of aqueous ferrocyanide solutions by the fourth harmonic of a mode locked Nd³⁺ laser. The rate of formation of the localized hydrated electron is ≈ 2 psec.

Original language	English
Pages (from-to)	480-482
Number of pages	3
Journal	Chemical Physics Letters
Volume	15
Issue number	4
DOIs	https://doi.org/10.1016/0009-2614(72)80353-1
State	Published - 1 Sep 1972

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title = "Relaxation of excess electrons in a polar solvent",

abstract = "We report the observation of the ultrafast relaxation of a quasifree electron to the localized excess electron state in water. Quasifree electrons were generated by photoionization of aqueous ferrocyanide solutions by the fourth harmonic of a mode locked Nd3+ laser. The rate of formation of the localized hydrated electron is ≈ 2 psec.",

author = "Rentzepis, {P. M.} and Jones, {R. P.} and Joshua Jortner",

year = "1972",

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N2 - We report the observation of the ultrafast relaxation of a quasifree electron to the localized excess electron state in water. Quasifree electrons were generated by photoionization of aqueous ferrocyanide solutions by the fourth harmonic of a mode locked Nd3+ laser. The rate of formation of the localized hydrated electron is ≈ 2 psec.

AB - We report the observation of the ultrafast relaxation of a quasifree electron to the localized excess electron state in water. Quasifree electrons were generated by photoionization of aqueous ferrocyanide solutions by the fourth harmonic of a mode locked Nd3+ laser. The rate of formation of the localized hydrated electron is ≈ 2 psec.

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JO - Chemical Physics Letters

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Relaxation of excess electrons in a polar solvent

Abstract

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