TY - JOUR
T1 - Predictive Semiclassical Model for Coherent and Incoherent Emission in the Strong Field Regime
T2 - The Mollow Triplet Revisited
AU - Chen, Hsing Ta
AU - Li, Tao E.
AU - Nitzan, Abraham
AU - Subotnik, Joseph E.
N1 - Publisher Copyright:
© 2019 American Chemical Society.
PY - 2019/3/21
Y1 - 2019/3/21
N2 - We reinvestigate the famous Mollow triplet and show that most of the well-known quantum characteristics of the Mollow triplet - including incoherent emission and a nonstandard dependence of the sidebands on detuning - can be recovered quantitatively using semiclassical dynamics with a classical light field. In fact, by not relying on the rotating wave approximation, a semiclassical model predicts some quantum effects beyond the quantum optical Bloch equation, including higher-order scattering and asymmetric sideband features. This Letter highlights the fact that, with strong intensities, many putatively quantum features of light-matter interactions arise from a simple balance of mean-field electrodynamics and elementary spontaneous emission, which requires minimal computational cost. Our results suggest that the application of semiclassical electrodynamics to problems with strong light-matter coupling in the fields of nanophotonics and superradiance are likely to yield a plethora of new information.
AB - We reinvestigate the famous Mollow triplet and show that most of the well-known quantum characteristics of the Mollow triplet - including incoherent emission and a nonstandard dependence of the sidebands on detuning - can be recovered quantitatively using semiclassical dynamics with a classical light field. In fact, by not relying on the rotating wave approximation, a semiclassical model predicts some quantum effects beyond the quantum optical Bloch equation, including higher-order scattering and asymmetric sideband features. This Letter highlights the fact that, with strong intensities, many putatively quantum features of light-matter interactions arise from a simple balance of mean-field electrodynamics and elementary spontaneous emission, which requires minimal computational cost. Our results suggest that the application of semiclassical electrodynamics to problems with strong light-matter coupling in the fields of nanophotonics and superradiance are likely to yield a plethora of new information.
UR - http://www.scopus.com/inward/record.url?scp=85063149919&partnerID=8YFLogxK
U2 - 10.1021/acs.jpclett.9b00181
DO - 10.1021/acs.jpclett.9b00181
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AN - SCOPUS:85063149919
SN - 1948-7185
VL - 10
SP - 1331
EP - 1336
JO - Journal of Physical Chemistry Letters
JF - Journal of Physical Chemistry Letters
IS - 6
ER -