Nonvanishing Subgap Photocurrent as a Probe of Lifetime Effects

Daniel Kaplan, Tobias Holder*, Binghai Yan

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

20 Scopus citations

Abstract

For semiconductors and insulators, it is commonly believed that in-gap transitions into nonlocalized states are smoothly suppressed in the clean limit; i.e., at zero temperature, their contribution vanishes due to the unavailability of states. We present a novel type of subgap response which shows that this intuition does not generalize beyond linear response. Namely, we find that the dc current due to the bulk photovoltaic effect can be finite and mostly temperature independent in an allowed window of subgap transitions. We expect that a moderate range of excitation energies lies between the bulk energy gap and the mobility edge where this effect is observable. Using a simplified relaxation time model for the band broadening, we find the subgap dc current to be temperature independent for noninteracting systems but temperature dependent for strongly interacting systems. Thus, the subgap response may be used to distinguish whether a state is single-particle localized or many-body localized.

Original languageEnglish
Article number227205
JournalPhysical Review Letters
Volume125
Issue number22
DOIs
StatePublished - 25 Nov 2020
Externally publishedYes

Funding

FundersFunder number
European Union’s Horizon 2020 research and innovation program
Willner Family Leadership Institute for the Weizmann Institute of Science
Horizon 2020 Framework Programme815869
European Research Council

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