Nonlinear relaxation and solvation dynamics in a Coulomb lattice gas

D. Knödler; W. Dieterich; C. Lonsky; A. Nitzan

doi:10.1063/1.469424

Nonlinear relaxation and solvation dynamics in a Coulomb lattice gas

D. Knödler^*, W. Dieterich, C. Lonsky, A. Nitzan

^*Corresponding author for this work

School of Chemistry

University of Konstanz

Research output: Contribution to journal › Article › peer-review

4 Scopus citations

Abstract

The transient response of ions upon sudden creation or removal of a local, external charge in a one-component Coulomb lattice gas is investigated by Monte Carlo simulations. Our model can be regarded as a simplified description of solvation dynamics processes in electrolyte systems. Effects of the nonlinearity of the relaxation are pointed out and are contrasted with predictions from linear (Debye-Hückel and Debye-Falkenhagen) theories.

Original language	English
Pages (from-to)	465-470
Number of pages	6
Journal	The Journal of Chemical Physics
Volume	102
Issue number	1
DOIs	https://doi.org/10.1063/1.469424
State	Published - 1995

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abstract = "The transient response of ions upon sudden creation or removal of a local, external charge in a one-component Coulomb lattice gas is investigated by Monte Carlo simulations. Our model can be regarded as a simplified description of solvation dynamics processes in electrolyte systems. Effects of the nonlinearity of the relaxation are pointed out and are contrasted with predictions from linear (Debye-H{\"u}ckel and Debye-Falkenhagen) theories.",

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AB - The transient response of ions upon sudden creation or removal of a local, external charge in a one-component Coulomb lattice gas is investigated by Monte Carlo simulations. Our model can be regarded as a simplified description of solvation dynamics processes in electrolyte systems. Effects of the nonlinearity of the relaxation are pointed out and are contrasted with predictions from linear (Debye-Hückel and Debye-Falkenhagen) theories.

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Nonlinear relaxation and solvation dynamics in a Coulomb lattice gas

Abstract

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