Nonlinear laser spectroscopy of nonlinear solvation

B. D. Fainberg, B. Zolotov, D. Huppert

Research output: Contribution to journalArticlepeer-review

Abstract

In this study we show that the transient four-photon spectroscopy with pulses longer than the electronic transition dephasing can be used for nonlinear solvation study, i.e., when the linear response for the solvation dynamics breaks down. We have obtained new formulae describing the time evolution of the moments of the nonlinear optical spectra and, in particular, the time resolved fluorescence in the case of nonlinear solvation.

Original languageEnglish
Pages (from-to)789-807
Number of pages19
JournalJournal of Nonlinear Optical Physics and Materials
Volume5
Issue number4
DOIs
StatePublished - Oct 1996

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