Nonlinear laser spectroscopy of nonlinear solvation

B. D. Fainberg*, B. Zolotov, D. Huppert

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review


In this study we show that the transient four-photon spectroscopy with pulses longer than the electronic transition dephasing can be used for nonlinear solvation study, i.e., when the linear response for the solvation dynamics breaks down. We have obtained new formulae describing the time evolution of the moments of the nonlinear optical spectra and, in particular, the time resolved fluorescence in the case of nonlinear solvation.

Original languageEnglish
Pages (from-to)789-807
Number of pages19
JournalJournal of Nonlinear Optical Physics and Materials
Issue number4
StatePublished - Oct 1996


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