@article{4f4213ec00ae456da8b9e3f55acb1214,
title = "Multi-channel electronic and vibrational dynamics in polyatomic resonant high-order harmonic generation",
abstract = "High-order harmonic generation in polyatomic molecules generally involves multiple channels of ionization. Their relative contribution can be strongly influenced by the presence of resonances, whose assignment remains a major challenge for high-harmonic spectroscopy. Here we present a multi-modal approach for the investigation of unaligned polyatomic molecules, using SF6 as an example. We combine methods from extreme-ultraviolet spectroscopy, above-threshold ionization and attosecond metrology. Fragment-resolved above-threshold ionization measurements reveal that strong-field ionization opens at least three channels. A shape resonance in one of them is found to dominate the signal in the 20-26 eV range. This resonance induces a phase jump in the harmonic emission, a switch in the polarization state and different dynamical responses to molecular vibrations. This study demonstrates a method for extending high-harmonic spectroscopy to polyatomic molecules, where complex attosecond dynamics are expected.",
author = "A. Ferr{\'e} and Boguslavskiy, {A. E.} and M. Dagan and V. Blanchet and Bruner, {B. D.} and F. Burgy and A. Camper and D. Descamps and B. Fabre and N. Fedorov and J. Gaudin and G. Geoffroy and J. Mikosch and S. Patchkovskii and S. Petit and T. Ruchon and H. Soifer and D. Staedter and I. Wilkinson and A. Stolow and N. Dudovich and Y. Mairesse",
note = "Publisher Copyright: {\textcopyright} 2015 Macmillan Publishers Limited. All rights reserved.",
year = "2015",
month = jan,
day = "22",
doi = "10.1038/ncomms6952",
language = "אנגלית",
volume = "6",
journal = "Nature Communications",
issn = "2041-1723",
publisher = "Nature Research",
}