TY - JOUR
T1 - Langevin-bloch equations for a spin bath
AU - Ghosh, Arnab
AU - Sinha, Sudarson Sekhar
AU - Ray, Deb Shankar
N1 - Funding Information:
Thanks are due to the Council of Scientific and Industrial Research, Government of India for partial financial support.
PY - 2011/3/7
Y1 - 2011/3/7
N2 - We derive the Bloch equations for a two-level system coupled to a spin bath of infinitely many two-level atoms to examine phase and energy relaxation of an optically excited system. We show that increasing temperature assists coherence. This is reflected in a number of anomalous features of relaxation of the system, e.g., decrease of integrated absorption coefficient with temperature, nonlinear variation of linewidth with incident power. We also predict that thermally induced coherence may result in anomalous narrowing of linewidth, reminiscent (but distinct) of motional narrowing of spectral line. The theoretical results are discussed in the light of absorption-emission experiments on single quantum dots.
AB - We derive the Bloch equations for a two-level system coupled to a spin bath of infinitely many two-level atoms to examine phase and energy relaxation of an optically excited system. We show that increasing temperature assists coherence. This is reflected in a number of anomalous features of relaxation of the system, e.g., decrease of integrated absorption coefficient with temperature, nonlinear variation of linewidth with incident power. We also predict that thermally induced coherence may result in anomalous narrowing of linewidth, reminiscent (but distinct) of motional narrowing of spectral line. The theoretical results are discussed in the light of absorption-emission experiments on single quantum dots.
UR - http://www.scopus.com/inward/record.url?scp=79952519548&partnerID=8YFLogxK
U2 - 10.1063/1.3556706
DO - 10.1063/1.3556706
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C2 - 21384957
AN - SCOPUS:79952519548
SN - 0021-9606
VL - 134
JO - Journal of Chemical Physics
JF - Journal of Chemical Physics
IS - 9
M1 - 094114
ER -