High-order optical harmonic generation on carbon nanotubes: Quantum-mechanical approach

G. Ya Slepyan; A. A. Khrutchinskii; A. M. Nemilentsau; S. A. Maksimenko; J. Herrmann

doi:10.1142/S0219581X04002152

High-order optical harmonic generation on carbon nanotubes: Quantum-mechanical approach

G. Ya Slepyan^*, A. A. Khrutchinskii, A. M. Nemilentsau, S. A. Maksimenko, J. Herrmann

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

Abstract

The high harmonic generation by a single-wall carbon nanotube (CNT) due to the interaction with femtosecond laser pulses is investigated. The analysis utilizes the quantum kinetic equations for π-electrons with both intra-band and inter-band transitions. Nonperturbative approach using numerical solution of the quantum kinetic equations in the time domain has been developed and the density of the axial electric current in CNT has been calculated. The amplitude of this current and the conversion efficiency in dependence on the number of the high-order harmonics, the CNT type, the frequency and the intensity of the driving field have been investigated.

Original language	English
Pages (from-to)	343-354
Number of pages	12
Journal	International Journal of Nanoscience
Volume	3
Issue number	3
DOIs	https://doi.org/10.1142/S0219581X04002152
State	Published - Jun 2004
Externally published	Yes

Keywords

Harmonic
Nanotube
Spectrum

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10.1142/S0219581X04002152

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title = "High-order optical harmonic generation on carbon nanotubes: Quantum-mechanical approach",

abstract = "The high harmonic generation by a single-wall carbon nanotube (CNT) due to the interaction with femtosecond laser pulses is investigated. The analysis utilizes the quantum kinetic equations for π-electrons with both intra-band and inter-band transitions. Nonperturbative approach using numerical solution of the quantum kinetic equations in the time domain has been developed and the density of the axial electric current in CNT has been calculated. The amplitude of this current and the conversion efficiency in dependence on the number of the high-order harmonics, the CNT type, the frequency and the intensity of the driving field have been investigated.",

keywords = "Harmonic, Nanotube, Spectrum",

author = "Slepyan, {G. Ya} and Khrutchinskii, {A. A.} and Nemilentsau, {A. M.} and Maksimenko, {S. A.} and J. Herrmann",

note = "Funding Information: The research was partially supported by the BMBF under Project No. BEL-001-01, INTAS under project No. 03-50-4409 and from the Belarus Foundation for Fundamental Research under Project Nos. F02-176 and F02R-047. A. M. Nemilentsau acknowledges the support from the World Federation of Scientists, Scholarship Programme.",

year = "2004",

month = jun,

doi = "10.1142/S0219581X04002152",

language = "אנגלית",

volume = "3",

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journal = "International Journal of Nanoscience",

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AU - Khrutchinskii, A. A.

AU - Nemilentsau, A. M.

AU - Maksimenko, S. A.

AU - Herrmann, J.

N1 - Funding Information: The research was partially supported by the BMBF under Project No. BEL-001-01, INTAS under project No. 03-50-4409 and from the Belarus Foundation for Fundamental Research under Project Nos. F02-176 and F02R-047. A. M. Nemilentsau acknowledges the support from the World Federation of Scientists, Scholarship Programme.

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N2 - The high harmonic generation by a single-wall carbon nanotube (CNT) due to the interaction with femtosecond laser pulses is investigated. The analysis utilizes the quantum kinetic equations for π-electrons with both intra-band and inter-band transitions. Nonperturbative approach using numerical solution of the quantum kinetic equations in the time domain has been developed and the density of the axial electric current in CNT has been calculated. The amplitude of this current and the conversion efficiency in dependence on the number of the high-order harmonics, the CNT type, the frequency and the intensity of the driving field have been investigated.

AB - The high harmonic generation by a single-wall carbon nanotube (CNT) due to the interaction with femtosecond laser pulses is investigated. The analysis utilizes the quantum kinetic equations for π-electrons with both intra-band and inter-band transitions. Nonperturbative approach using numerical solution of the quantum kinetic equations in the time domain has been developed and the density of the axial electric current in CNT has been calculated. The amplitude of this current and the conversion efficiency in dependence on the number of the high-order harmonics, the CNT type, the frequency and the intensity of the driving field have been investigated.

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KW - Nanotube

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High-order optical harmonic generation on carbon nanotubes: Quantum-mechanical approach

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Keywords

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