First-principles investigation of morphotropic transitions and phase-change functional responses in BiFeO3-BiCoO3 multiferroic solid solutions

Oswaldo Diéguez*, Jorge Añiguez

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

87 Scopus citations

Abstract

We present an ab initio study of the BFCO solid solution formed by multiferroics BiFeO3 (BFO) and BiFeO3 (BCO). We find that BFCO presents a strongly discontinuous morphotropic transition between BFO-like and BCO-like ferroelectric phases. Further, for all compositions such phases remain (meta)stable and retain well-differentiated properties. Our results thus suggest that an electric field can be used to switch between these structures and show that such a switching involves large phase-change effects of various types, including piezoelectric, electric, and magnetoelectric ones.

Original languageEnglish
Article number057601
JournalPhysical Review Letters
Volume107
Issue number5
DOIs
StatePublished - 26 Jul 2011
Externally publishedYes

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