@article{da1328778a264176847d612230c465ae,
title = "Ehrenfest+R dynamics. II. A semiclassical QED framework for Raman scattering",
abstract = "In Paper I [Chen et al., J. Chem. Phys. 150, 044102 (2019)], we introduced Ehrenfest+R dynamics for a two-level system and showed how spontaneous emission can be heuristically included such that, after averaging over an ensemble of Ehrenfest+R trajectories, one can recover both coherent and incoherent electromagnetic fields. In the present paper, we now show that Ehrenfest+R dynamics can also correctly describe Raman scattering, whose features are completely absent from standard Ehrenfest dynamics. Ehrenfest+R dynamics appear to be quantitatively accurate both for resonant and off-resonant Raman signals, as compared with Kramers-Heisenberg-Dirac theory.",
author = "Chen, \{Hsing Ta\} and Li, \{Tao E.\} and Maxim Sukharev and Abraham Nitzan and Subotnik, \{Joseph E.\}",
note = "Publisher Copyright: {\textcopyright} 2019 Author(s).",
year = "2019",
month = jan,
day = "28",
doi = "10.1063/1.5057366",
language = "אנגלית",
volume = "150",
journal = "Journal of Chemical Physics",
issn = "0021-9606",
publisher = "American Institute of Physics",
number = "4",
}