Effect of NO, CO, and Cl2 on mixed-mode regimes in the Belousov-Zhabotinskyi oscillating chemical reaction in a CSTR

Peter E. Strizhak; Vyacheslav O. Khavrus; Kedma Bar-Eli

doi:10.1021/jp011774k

Effect of NO, CO, and Cl₂ on mixed-mode regimes in the Belousov-Zhabotinskyi oscillating chemical reaction in a CSTR

Peter E. Strizhak^*
, Vyacheslav O. Khavrus
, Kedma Bar-Eli

^*Corresponding author for this work

School of Chemistry

National Academy of Sciences of Ukraine

Research output: Contribution to journal › Article › peer-review

6 Scopus citations

Abstract

We have studied the effect of gases (NO, CO, Cl₂) on mixed-mode regimes in the Belousov-Zhabotinskyi oscillating chemical reaction in a CSTR. Mixed-mode regimes are characterized by a single large-amplitude oscillation followed by a number of small-amplitude oscillations. Bubbling of the gas into the inflow solution changes the average number of small-amplitude oscillations. We show that the average number of small-amplitude oscillations depends linearly on the gas concentration. A good agreement between the experimental data and simulations with the Györgyi-Field model is obtained.

Original language	English
Pages (from-to)	2505-2511
Number of pages	7
Journal	Journal of Physical Chemistry A
Volume	106
Issue number	11
DOIs	https://doi.org/10.1021/jp011774k
State	Published - 21 Mar 2002

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title = "Effect of NO, CO, and Cl2 on mixed-mode regimes in the Belousov-Zhabotinskyi oscillating chemical reaction in a CSTR",

abstract = "We have studied the effect of gases (NO, CO, Cl2) on mixed-mode regimes in the Belousov-Zhabotinskyi oscillating chemical reaction in a CSTR. Mixed-mode regimes are characterized by a single large-amplitude oscillation followed by a number of small-amplitude oscillations. Bubbling of the gas into the inflow solution changes the average number of small-amplitude oscillations. We show that the average number of small-amplitude oscillations depends linearly on the gas concentration. A good agreement between the experimental data and simulations with the Gy{\"o}rgyi-Field model is obtained.",

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T1 - Effect of NO, CO, and Cl2 on mixed-mode regimes in the Belousov-Zhabotinskyi oscillating chemical reaction in a CSTR

AU - Strizhak, Peter E.

AU - Khavrus, Vyacheslav O.

AU - Bar-Eli, Kedma

PY - 2002/3/21

Y1 - 2002/3/21

N2 - We have studied the effect of gases (NO, CO, Cl2) on mixed-mode regimes in the Belousov-Zhabotinskyi oscillating chemical reaction in a CSTR. Mixed-mode regimes are characterized by a single large-amplitude oscillation followed by a number of small-amplitude oscillations. Bubbling of the gas into the inflow solution changes the average number of small-amplitude oscillations. We show that the average number of small-amplitude oscillations depends linearly on the gas concentration. A good agreement between the experimental data and simulations with the Györgyi-Field model is obtained.

AB - We have studied the effect of gases (NO, CO, Cl2) on mixed-mode regimes in the Belousov-Zhabotinskyi oscillating chemical reaction in a CSTR. Mixed-mode regimes are characterized by a single large-amplitude oscillation followed by a number of small-amplitude oscillations. Bubbling of the gas into the inflow solution changes the average number of small-amplitude oscillations. We show that the average number of small-amplitude oscillations depends linearly on the gas concentration. A good agreement between the experimental data and simulations with the Györgyi-Field model is obtained.

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U2 - 10.1021/jp011774k

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SN - 1089-5639

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JO - Journal of Physical Chemistry A

JF - Journal of Physical Chemistry A

IS - 11

ER -

Effect of NO, CO, and Cl₂ on mixed-mode regimes in the Belousov-Zhabotinskyi oscillating chemical reaction in a CSTR

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